{"id":704,"date":"2024-04-26T12:46:30","date_gmt":"2024-04-26T19:46:30","guid":{"rendered":"https:\/\/dornsife.usc.edu\/stephen-bradforth\/?p=704"},"modified":"2024-04-26T12:56:15","modified_gmt":"2024-04-26T19:56:15","slug":"704","status":"publish","type":"post","link":"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/","title":{"rendered":"Indole Photoionization and Coinage Metal CMA Photosensitizer Publications Accepted!"},"content":{"rendered":"\n\n\n        \n  \n    \n\n\n\n\n\n\n<div\n  class=\"cc--component-container cc--image-gallery \"\n\n  \n  \n  \n  \n  \n  \n  >\n  <div class=\"c--component c--image-gallery\"\n    \n      >\n\n    \n  <div class=\"inner-wrapper\">\n\n    \n      <div id=\"gallery-877536608\" class=\"gallery-container\">\n\n      <div class=\"swiper images\">\n        <div class=\"swiper-wrapper\">\n                                    <div class=\"swiper-slide\">\n                                      \n<div class=\"f--field f--image\">\n\n    \n    \n    \n    \n    \n    \n              \n      <img\n                            data-src=\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/wp-content\/uploads\/sites\/416\/2024\/04\/images_large_jp4c01994_0012.jpeg\"\n                    data-sizes=\"(min-width:1200px) 75vw, (min-width:768px) 83vw, 100vw\"          class=\"lazyload\"\n        \n                  role=\"none\"\n        \n        \n                                      \/>\n\n    \n    \n  \n  \n\n<\/div>\n                              <\/div>\n                                                <div class=\"swiper-slide\">\n                                      \n<div class=\"f--field f--image\">\n\n    \n    \n    \n    \n    \n    \n              \n      <img\n                            data-src=\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/wp-content\/uploads\/sites\/416\/2024\/04\/jp4c01223_0007.webp\"\n                    data-sizes=\"(min-width:1200px) 75vw, (min-width:768px) 83vw, 100vw\"          class=\"lazyload\"\n        \n                  role=\"none\"\n        \n        \n                                      \/>\n\n    \n    \n  \n  \n\n<\/div>\n                              <\/div>\n                              <\/div>\n      <\/div>\n\n      <div class=\"swiper captions\">\n        <div class=\"controls-container\">\n          <button class=\"button-prev\" aria-label=\"Previous Image\">\n            <svg version=\"1.1\" xmlns=\"http:\/\/www.w3.org\/2000\/svg\" xmlns:xlink=\"http:\/\/www.w3.org\/1999\/xlink\"\n            x=\"0px\" y=\"0px\" viewBox=\"0 0 35 35\" enable-background=\"new 0 0 35 35\" xml:space=\"preserve\">\n            <polygon fill-rule=\"evenodd\" clip-rule=\"evenodd\" fill=\"#000\" points=\"15.7,27.5 5.7,17.5 \n            15.7,7.5 18.7,10.4 13.6,15.4 28.3,15.4 28.3,19.6 13.6,19.6 18.7,24.6 \"\/>\n            <\/svg>\n          <\/button>\n          <button class=\"button-next\" aria-label=\"Next Image\">\n            <svg version=\"1.1\" xmlns=\"http:\/\/www.w3.org\/2000\/svg\" xmlns:xlink=\"http:\/\/www.w3.org\/1999\/xlink\"\n\t x=\"0px\" y=\"0px\" viewBox=\"0 0 35 35\" enable-background=\"new 0 0 35 35\" xml:space=\"preserve\"><polygon fill-rule=\"evenodd\" clip-rule=\"evenodd\" fill=\"#000\" points=\"19.3,27.5 29.3,17.5 \n\t19.3,7.5 16.3,10.4 21.4,15.4 6.7,15.4 6.7,19.6 21.4,19.6 16.3,24.6 \"\/>\n<\/svg>\n          <\/button>\n        <\/div>\n\n        <div class=\"swiper-wrapper\">\n                                    <div class=\"swiper-slide\">\n                                  <div class=\"slide-caption\">\n                        \n<div class=\"f--field f--description\">\n\n    \n  <p>Using time-correlated single photon counting (TCSPC) and psTA with a thermally activated delayed fluorescence (TADF) model, the variation in intersystem crossing (ISC), (S1 \u2192 T1) rates (\u223c3\u2013120 \u00d7 109 s\u20131), and \u0394EST values (73\u2013115 meV) for the Carbazole-Metal-Amide compounds were fully characterized, reflecting systematic changes to the carbene, carbazole, and metal.<\/p>\n\n\n\n<\/div>\n                  <\/div>\n                              <\/div>\n                                                <div class=\"swiper-slide\">\n                                  <div class=\"slide-caption\">\n                        \n<div class=\"f--field f--description\">\n\n    \n  <p>The photoionization dynamics of indole, the ultraviolet-B chromophore of tryptophan, were explored in water and ethanol using ultrafast transient absorption spectroscopy with 292, 268, and 200 nm excitation.<\/p>\n\n\n\n<\/div>\n                  <\/div>\n                              <\/div>\n                              <\/div>\n\n      <\/div>\n\n\n    <\/div>\n  \n  <\/div>\n\n\n  <\/div><\/div>\n\n\n  \n    \n\n\n\n\n\n\n<div\n  class=\"cc--component-container cc--article-intro \"\n\n  \n  \n  \n  \n  \n  \n  >\n  <div class=\"c--component c--article-intro\"\n    \n      >\n\n    \n          \n<div class=\"f--field f--description\">\n\n    \n  <p>Two important papers published this week by the Bradforth group. Take a look at the full list of the group\u2019s publications which are now searchable by tags.  (As with our recent JACS paper, both are open access and also have data deposited in an open access repository)<\/p>\n<p>The <a href=\"https:\/\/pubs.acs.org\/doi\/10.1021\/acs.jpcc.4c01994\">first paper<\/a> provides a full spectroscopic journey for light conversion by a carbene-metal-amide (cMa) photosensitizers based on coinage metals. This appears in a virtual special issue on thermally assisted delayed fluorescence (TADF) active systems in the Journal of Physical Chemistry C. Using transient absorption over 9 decades in time we follow the relaxation of a ligand-to-ligand charge transfer state excited with a femtosecond pulse, all the way out to transferring the separated charges to electron and hole acceptors in homogeneous solution.  In a collaboration with Mark Thompson\u2019s group at USC and Matt Bird at Brookhaven National Lab, we show the effect of changing central metal and the carbene and carbazole ligands and what it reveals the spin-orbit coupling and singlet-triplet energy gaps in these TADF chromophores.  The photostability of certain cMa complexes are demonstrated and photosensitizers based on gold have been shown to produce hydrogen under visible light irradiation.<\/p>\n<p>The <a href=\"https:\/\/pubs.acs.org\/doi\/full\/10.1021\/acs.jpcb.4c01223\">second paper<\/a>, titled \u201cUnraveling the Photoionization Dynamics of Indole in Aqueous and Ethanol Solutions\u201d represents a Herculean effort to fully understand the photodynamics of the intrinsic protein chromophore in tryptophan.  Tryptophan fluorescence is routinely studied in biophysical assays and microscopy and the lifetime is known to be sensitive to the local environment, particularly water exposure. But what initially seems simple, a changing quantum yield in water, turns out to reflect rather complex photoionization dynamics that are specific to an aqueous environment.  Tom Oliver at the University of Bristol was central to unravelling this problem.  Tom will be a sabbatical visitor in the group from October.<\/p>\n\n\n\n<\/div>\n  \n\n  <\/div><\/div>\n","protected":false},"excerpt":{"rendered":"","protected":false},"author":752,"featured_media":706,"comment_status":"open","ping_status":"open","sticky":false,"template":"","format":"standard","meta":{"_acf_changed":false,"footnotes":""},"categories":[10],"tags":[],"class_list":["post-704","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-newly-published"],"acf":[],"yoast_head":"<!-- This site is optimized with the Yoast SEO plugin v27.1.1 - https:\/\/yoast.com\/product\/yoast-seo-wordpress\/ -->\n<title>Indole Photoionization and Coinage Metal CMA Photosensitizer Publications Accepted!<\/title>\n<meta name=\"robots\" content=\"index, follow, max-snippet:-1, max-image-preview:large, max-video-preview:-1\" \/>\n<link rel=\"canonical\" href=\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\" \/>\n<meta property=\"og:locale\" content=\"en_US\" \/>\n<meta property=\"og:type\" content=\"article\" \/>\n<meta property=\"og:title\" content=\"Indole Photoionization and Coinage Metal CMA Photosensitizer Publications Accepted! - Bradforth Research Group\" \/>\n<meta property=\"og:url\" content=\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\" \/>\n<meta property=\"og:site_name\" content=\"Bradforth Research Group\" \/>\n<meta property=\"article:published_time\" content=\"2024-04-26T19:46:30+00:00\" \/>\n<meta property=\"article:modified_time\" content=\"2024-04-26T19:56:15+00:00\" \/>\n<meta property=\"og:image\" content=\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/wp-content\/uploads\/sites\/416\/2024\/04\/jp4c01223_0007.webp\" \/>\n\t<meta property=\"og:image:width\" content=\"500\" \/>\n\t<meta property=\"og:image:height\" content=\"304\" \/>\n\t<meta property=\"og:image:type\" content=\"image\/webp\" \/>\n<meta name=\"author\" content=\"Brandon Young\" \/>\n<meta name=\"twitter:card\" content=\"summary_large_image\" \/>\n<script type=\"application\/ld+json\" class=\"yoast-schema-graph\">{\"@context\":\"https:\/\/schema.org\",\"@graph\":[{\"@type\":\"Article\",\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/#article\",\"isPartOf\":{\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\"},\"author\":{\"name\":\"Brandon Young\",\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/#\/schema\/person\/db05f5e4e5af6c03394c4b49f8dc846b\"},\"headline\":\"Indole Photoionization and Coinage Metal CMA Photosensitizer Publications Accepted!\",\"datePublished\":\"2024-04-26T19:46:30+00:00\",\"dateModified\":\"2024-04-26T19:56:15+00:00\",\"mainEntityOfPage\":{\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\"},\"wordCount\":9,\"commentCount\":0,\"image\":{\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/#primaryimage\"},\"thumbnailUrl\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/wp-content\/uploads\/sites\/416\/2024\/04\/jp4c01223_0007.webp\",\"articleSection\":[\"Newly Published\"],\"inLanguage\":\"en-US\",\"potentialAction\":[{\"@type\":\"CommentAction\",\"name\":\"Comment\",\"target\":[\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/#respond\"]}]},{\"@type\":\"WebPage\",\"@id\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\",\"url\":\"https:\/\/dornsife.usc.edu\/stephen-bradforth\/2024\/04\/26\/704\/\",\"name\":\"Indole Photoionization and Coinage Metal CMA Photosensitizer Publications Accepted! 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